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Unraveling an Alternative Mechanism in Polymer Self-Assemblies : An Order-Order Transition with Unusual Molecular Interactions between Hydrophilic and Hydrophobic Polymer Blocks

Hahn, Lukas; Zorn, Theresa; Kehrein, Josef; Kielholz, Tobias; Ziegler, Anna Lena; Forster, Stefan; Sochor, Benedikt; Lisitsyna, Ekaterina S.; Durandin, Nikita A.; Laaksonen, Timo; Aseyev, Vladimir; Sotriffer, Christoph; Saalwächter, Kay; Windbergs, Maike; Pöppler, Ann Christin; Luxenhofer, Robert (2023)
article

Polymer self-assembly leading to cooling-induced hydrogel formation is relatively rare for synthetic polymers and typically relies on H-bonding between repeat units. Here, we describe a non-H-bonding mechanism for a ...